iPhone iSync is potentially a very interesting application with great promise. It’s a GUI implementation of an rsync-based folder synchronization tool that works with WiFi. This means it will sync a folder on your Mac to your iPhone/iPod touch over the wireless network. In the future, this suggests the possibility of iTunes syncing over WiFi… unfortunately, it’s not quite there yet.

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The author, francisois, says that he has “reached a breakthrough that has allowed me to synchronize my own iPod Touch over wi-fi with an older version of iTunes,” and he is working on getting iTunes 7.5 support but a few obstacles remain. Nonetheless, he eventually plans for syncing music, photos, contacts, and bookmarks over WiFi.

Obviously you’ll need a jailbroken iPhone to use this. If you have any experience with “shell scripts and ssh and especially iTunes library access,” francisois is looking for help. iPhone iSync is a free download from its Google Code page.

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